PSILOGO

Laboratory for Particle Physics (LTP)


LTP Colloquium

Analytic Progress in Accelerator Mass Spectrometry and related Opportunities for Applications with long-lived Radionuclides

Thursday, December 2, 2021, 16:00
online only                                             (for the zoom link contact michael.spira@psi.ch, johannes.schlenk@psi.ch or antonio.coutinho@psi.ch)

Hans-Arno Synal, ETHZ

Abstract:
The Laboratory of Ion Beam Physics (LIP) provides a world class infrastructure for accelerator mass spectrometry (AMS) and serves as a national and international center for radiocarbon dating, and applications of isotopes as clocks or tracers in environmental, climate, astrophysical, or pharmaceutical studies. Over the last ten years, we have improved AMS measurement technology based on fundamental research to enable ultra-sensitive and background free detection of radionuclides. In the case of radiocarbon, which is still the most important radionuclide in AMS, measurement technology has now reached a stage, where almost tabletop instrumentation (MICADAS) provides high overall detection efficiency, reach highly reproducible measurement conditions, and can be operated by trained lab technicians. This became possible because molecular interferences, the dominant interfering background, can be destroyed in multiple collisions with He stripper gas atoms and utilizing 1+ charge state. The advent of hybrid ion source accepting sample materials as CO2 in a He carrier gas stream enabled the analysis of microgram sized samples making compound specific analyses possible and opening new application fields. He stripping has the potential to down size instruments for measurements of other radionuclides, too. In collaboration of ETH Zurich and the Ionplus AG, a Multi-Isotope-Low-Energy-AMS system (MILEA) has been developed based a small accelerator operating at only 0.3 MV. It has been shown that such a system can cover the analytic need for the detection of the most important AMS nuclides: 10Be, 14C, 26Al, 41Ca, 129I, and actinides. In fact, they reach the highest transmission of any AMS system for actinides. The recent technical development will be summarized and examples on specific applications will be discussed to highlight future perspective of research with long-lived radionuclides.